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Abstract
Layered transition metal chalcogenides are promising hosts of electronic Weyl nodes and topological superconductivity. MoTe2 is a striking example that harbors both noncentrosymmetric Td and centrosymmetric T’ phases, both of which have been identified as topologically nontrivial. Applied pressure tunes the structural transition separating these phases to zero temperature, stabilizing a mixed Td–T’ matrix that entails a network of interfaces between the two nontrivial topological phases. Here, we show that this critical pressure range is characterized by distinct coherent quantum oscillations, indicating that the difference in topology between topologically nonvtrivial Td and T’ phases gives rise to an emergent electronic structure: a network of topological interfaces. A rare combination of topologically nontrivial electronic structures and locked-in transformation barriers leads to this counterintuitive situation, wherein quantum oscillations can be observed in a structurally inhomogeneous material. These results further open the possibility of stabilizing multiple topological phases coexisting with superconductivity.
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1 NIST, NIST Center for Neutron Research, Gaithersburg, USA (GRID:grid.94225.38) (ISNI:000000012158463X); Department of Physics, University of Maryland, Center for Nanophysics and Advanced Materials, College Park, USA (GRID:grid.164295.d) (ISNI:0000 0001 0941 7177); University of Maryland, Department of Materials Science and Engineering, College Park, USA (GRID:grid.164295.d) (ISNI:0000 0001 0941 7177)
2 NIST, NIST Center for Neutron Research, Gaithersburg, USA (GRID:grid.94225.38) (ISNI:000000012158463X); NIST and University of Maryland, Joint Quantum Institute, College Park, USA (GRID:grid.164295.d) (ISNI:0000 0001 0941 7177)
3 NIST, NIST Center for Neutron Research, Gaithersburg, USA (GRID:grid.94225.38) (ISNI:000000012158463X)
4 Department of Physics, University of Maryland, Center for Nanophysics and Advanced Materials, College Park, USA (GRID:grid.164295.d) (ISNI:0000 0001 0941 7177)
5 NIST, NIST Center for Neutron Research, Gaithersburg, USA (GRID:grid.94225.38) (ISNI:000000012158463X); Department of Physics, University of Maryland, Center for Nanophysics and Advanced Materials, College Park, USA (GRID:grid.164295.d) (ISNI:0000 0001 0941 7177); University of Maryland, Department of Materials Science and Engineering, College Park, USA (GRID:grid.164295.d) (ISNI:0000 0001 0941 7177); Washington University in St. Louis, Department of Physics, St. Louis, USA (GRID:grid.4367.6) (ISNI:0000 0001 2355 7002)
6 NIST, NIST Center for Neutron Research, Gaithersburg, USA (GRID:grid.94225.38) (ISNI:000000012158463X); Department of Physics, University of Maryland, Center for Nanophysics and Advanced Materials, College Park, USA (GRID:grid.164295.d) (ISNI:0000 0001 0941 7177)