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Abstract
The exothermic heterogeneous electrochemical energy conversion to the electric energy through interaction of the ZrO2 based nanopowder system with atmospheric moisture have been explored within this work. Electrical properties of the experimental samples were investigated during humidification at the conditions of molecular flux density gradient. The morphological features of the surface cross-section and aggregates of 3 mol% Y2O3 doped ZrO2 nanopowder systems were investigated. Initial conditions for molecular dynamics modelling of the adsorption processes were obtained. A novel approach for developing of chemo-electronic converters based on nanoscale processes and materials with dielectric conductivity type proposed.
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1 Joint Institute for Nuclear Research, 141980, str. Joliot-Curie, 6, Dubna, Russia.; Donetsk Institute for Physics and Engineering named after O O Galkin NAS of Ukraine, 03680, Nauki ave, 46, Kyiv, Ukraine.
2 i3N/CENIMAT, Department of Materials Science, Faculty of Science and Technology, New University of Lisbon and CEMOP/UNINOVA, Campus de Caparica, 2829-516 Caparica, Portugal.
3 Joint Institute for Nuclear Research, 141980, str. Joliot-Curie, 6, Dubna, Russia.
4 Government Institution “Donetsk Institute for Physics and Engineering named after O O Galkin”, 83114, R. Luxembourg str., 72, Donetsk, Ukraine.
5 Dubna International University for Nature, Society and Man, 141980, st. Universitetskay, 19, Dubna, Moscow region, Russia.
6 Donetsk Institute for Physics and Engineering named after O O Galkin NAS of Ukraine, 03680, Nauki ave, 46, Kyiv, Ukraine.
7 Hiroshima Institute of Technology, Hiroshima 731-5193, Japan.
8 REQUIMTE, Chemical Department, Faculty of Science and Technology, New University of Lisbon, Campus de Caparica, 2829-516 Caparica, Portugal.
9 CQE-Centro de Química Estrutural, Instituto Superior Tecnico, Universidade de Lisboa, Av. Rovisco Pais 1, 1049-001 Lisbon, Portugal.
10 Institute of Semiconductor Physics NAS, Kiev, Ukraine, 03028, Nauki ave, 41, Kiev, Ukraine.
11 Joint Institute for Nuclear Research, 141980, str. Joliot-Curie, 6, Dubna, Russia.; Dubna International University for Nature, Society and Man, 141980, st. Universitetskay, 19, Dubna, Moscow region, Russia.