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Abstract
We measured the relative ionization delays into the two spin-orbit components of the electronic ground states of Xe+ and Kr+ under the inuence of auto-ionizing intermediate and final states. The results are in good agreement with state-of-the-art calculations based on the time-dependent configuration-interaction singles (TDCIS) approach.
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Details
1 Laboratory for physical chemistry, ETH Zurich, Vladimir-Prelog-Weg 2, CH-8093 Zurich, Switzerland
2 Center for Free-Electron Laser Science, DESY, Notkestrasse 85, 22607 Hamburg, Germany; ITAMP, Harvard-Smithsonian Center for Astrophysics, 60 Garden Street, Cambridge, MA 02138, USA