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1. Introduction
The interaction of charged particles with matter is an essential issue for a variety of physical systems, which has been a subject of extensive research since the discovery of subatomic particles [1]. Especially, the interests in surface physics are at the focus of much current research on charged particles interacting with two-dimensional (2D) electron gases [2–5]. Most intriguing is perhaps energy loss, i.e., so-called stopping power and the perturbed electron gas density induced by the charged particle in the interaction process [6–9]. Studying the stopping power of charged particle in dense plasmas is crucial for applications in high energy density physics [10, 11] and fundamental plasma physics [7, 12, 13], which can help us to make an accurate understanding of ion beam transport. Additionally, in ion beam analysis, where the stopping power of detected projectiles is the common observable quantity, the specific stopping power can obtain accurate depth perception [14]. Furthermore, the information given by the energy loss process in plasma is crucial for characterization and surface modification schemes [15–17] of the 2D system using projectiles in the matter as a powerful tool.
Stopping power is a measure of the ability of a material to slow down energetic particles that travel above the 2D sheet and 3D bulk [18]. When a charged particle moves with constant velocity near to a 2D sheet, the charged particle loses its kinetic energy, and the electron gas density of the 2D sheet is perturbed due to ionization and excitation of the electrons [19]. The stopping power, i.e., the energy lost per unit path length, is a substantial quantity used to predict and understand the effects of particle radiation in the matter, ion ranges, and the energy deposited [20–22]. There have been many works, both theoretical and experimental, investigating the stopping power [23–27]. Horing first investigated the energy loss of the fast particle moving parallel to the two-dimensional plasma sheet with a fixed distance by using the random-phase approximation (RPA) theory [28]. Apart from RPA theory, much work was carried out to study the stopping power by using the dielectric and binary collision theories [29–31], the quantum scattering theory [32], and the local field correction (LFC) [33, 34]. In addition, the density functional theory [35, 36], the first principles [18], and the particle-in-cell (PIC) and molecular dynamics (MD) [19, 37–38]were also adopted to study the interaction process between the ions and plasma. Recently, some progress has been made in the experimental study of the stopping power. J. Ren and coworkers [11] have performed an experiment to demonstrate the existence of collective effects, for high-density beam, leading to enhanced stopping. Their results play an important role in the optimum design of ion-driven inertial confinement fusion and fast ignition schemes. The importance of excited projectile states has been reported by Y. Zhao et al. [13] in the stopping process, providing significant support for the relevant research like the atomic process in the solar wind.
So far, with technological development in the area of miniaturized devices and the advances in nanofabrication techniques, plasmonic materials containing fully degenerated electrons have recently received renewed attention [39–42]. The quantum mechanical effects for the theoretical description of quantum plasma must be taken into account. For accurately understanding the dynamics of 2D quantum electron gas, the use of the quantum hydrodynamic model (QHD) is required, which was developed by solving the nonlinear Schrödinger–Poisson or the Wigner–Poisson kinetic models [43, 44]. Also, based on this model, both the quantum statistical and quantum diffraction effects have been proved to play an essential role in studying the interactions of charged particles with the quantum electron gas [45–48].
Interactions between particles in quantum many-body systems can bring about the collective behavior described by hydrodynamics. Some new features in the two-dimensional electron gas of the hydrodynamic regime will be produced on the condition that the typical length scale of electron-electron scattering
Recently, experiments on
However, to the best of our knowledge, viscosity in the two-dimensional quantum electron gas (2DQEG) effect has not been considered in beam-2DQEG interactions. Thus, an interesting question arises: How is the strength of the stopping power changed in the viscous 2D quantum electron gases? In this work, the main aim is to study the interaction between charged particles and 2D quantum electron gases in viscosity. We propose a revised quantum hydrodynamic model for a viscous two-dimensional quantum electron based on the model obtained in reference [64]. The outline of the study is as follows. In Section 2, we introduce our quantum hydrodynamic model and then derive the analytical expressions of the stopping power, the perturbed density, and the velocity vector field of perturbed electron gas based on revised QHD. In Section 3, numerical results of the perturbed density, spatial distribution of the velocity field, and the stopping power are discussed in different conditions. Moreover, we present the viscosity impacts on these quantities. Finally, a summary is given in Section 4. Gauss units will be adopted throughout the study.
2. Quantum Hydrodynamic Model
2.1. The Viscosity Coefficient
In the hydrodynamic regime, electronic dynamics is dominated by viscosity, rather than impurity scatting [56]. The electron flow in which numerous target nuclei are suspended (forming a suspension-like) may be regarded as a homogeneous medium. Such a medium has an effective viscosity
Consequently, as for
As a result, the corresponding viscosity
2.2. Derivation of the Fluid Model
We consider an idealized 2DEG with an equilibrium density,
[figure(s) omitted; refer to PDF]
By employing the linearized quantum hydrodynamic model of the incompressible viscous fluid, the electronic excitation on the 2DEG surface can be described by the continuity equation as
There is a weak perturbation in 2DEG by the moving charged particles. Hence, we can linearize the above equations by assuming the density, velocity field, and the potential written as
We adopt the time-space Fourier transform:
For convenience, we introduce the dimensionless variables:
The stopping power
Thus, we can obtain the expression of the dimensionless stopping power:
In the next section, the results of the perturbed electrons gas density, the velocity vector field of the perturbed electron gas, and the stopping power are obtained numerically according to (12), (14a), (14b), and (17), respectively, where the MATLAB solver function (integral2 function) is used to solve the double integral. Referring to [64] for parameter selection, we take the charge number of the incident particle is a proton
3. Numerical Results
3.1. The Perturbed Electron Density
We have solved (12) numerically for the values of the plasma configuration parameters
[figure(s) omitted; refer to PDF]
The comparison of the perturbed electron gas density for the different moving speeds (
[figure(s) omitted; refer to PDF]
3.2. The Spatial Distribution of the Velocity Vector Field
Figures 4 and 5 show the spatial distribution of the velocity vector field of perturbed electron gas for different incident particle speeds to further understand the influence of viscosity. We first show in Figures 4(a) and 4(b) the spatial distribution of the velocity vector field with
[figure(s) omitted; refer to PDF]
As demonstrated above, viscosity affects the spatial distribution and affects the maximum value of the velocity vector field. Thus, such a viscosity effect on the velocity vector of the perturbed electron gas
3.3. Stopping Power
The viscosity significantly impacts the density and velocity vector field of the perturbed electron gas. As a result, such an influence can also be seen in the stopping power, as shown in Figure 6, showing how the electronic stopping character is impacted by viscosity. The influence of viscosity is reflected clearly in Figure 6 where the stopping power is plotted as a function of velocity for the same condition shown in Figure 2. The main features observed in the perturbed density are reproduced in the stopping power. With the increasing
[figure(s) omitted; refer to PDF]
4. Summary
The purpose of this study was first to derive a self-consistent quantum hydrodynamic model that incorporates quantum and viscosity effects. Then, two-dimensional simulations are performed to investigate the interaction of the moving charged particle with 2DQEG, taking into account the viscosity based on the QHD model. Special attention is paid to the influences of the viscosity during interaction. The analytical expressions of the perturbed electron density, the velocity vector field in 2DQEG, and the stopping power have been derived based on the assumption of the linear disturbance. Results show that the viscosity effect suppresses the perturbation of the electron gas density and velocity vector field in the two-dimensional plane. As for considering the viscosity effect, our simulation results show that the oscillatory behaviors of the perturbed density and velocity vector field turn up in the case of small viscosity and then disappear gradually with the increasing of the viscosity. Besides, the magnitude of the wake-field decreases, and the perturbed regions caused by the moving particles get smaller due to the restriction on electron motion as the viscosity increases. The same trend is reproduced as the velocity of the incident particle increases. Furthermore, the perturbed density may change locally without changing in the surroundings due to the action of the viscous term [70]. The results indicate that the wake-field oscillation amplitude will decrease, and the incident particle will suffer less energy loss as the viscosity has been taken into account. Furthermore, in the stopping power calculation, the charged particle will suffer less energy loss.
In conclusion, viscosity not only affects the spatial distribution but also affects the magnitude. This is because the existence of the viscous term makes the electron gas less likely to be disturbed, resulting in the weakening of the electron polarization. In other words, due to the presence of a viscous effect, the average flow velocity of the electron gas is reduced, and the viscous flows may show a peculiar behavior that self-organizes into streams with different speeds. As a result, the distribution and magnitude of the disturbing electron gas are changed, giving rise to the reduction in the stopping power.
In summary, the model proposed in this study can be used in any system with two-dimensional electron gas such as the two-dimensional monovalent layered metal
Acknowledgments
This work was supported by the National Key R & D Program of China (2017YFE0301801), the National Natural Science Foundation of China (11975174 and 11775090), and the Fundamental Research Funds for the Central Universities (WUT: 2020IB023 and 2018IB011).
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Abstract
In two-dimensional (2D) electron systems, the viscous flow is dominant when electron-electron collisions occur more frequently than the impurity or phonon scattering. In this work, a quantum hydrodynamic model, considering viscosity, is proposed to investigate the interaction of a charged particle moving above the two-dimensional viscous electron gas. The stopping power, perturbed electron gas density, and the spatial distribution of the velocity vector field have been theoretically analyzed and numerically calculated. The calculation results show that viscosity affects the spatial distribution and amplitude of the velocity field. The stopping power, which is an essential quantity for describing the interactions of ions with the 2D electron gas, is calculated, indicating that the incident particle will suffer less energy loss due to the weakening of the dynamic electron polarization and induced electric field in 2D electron gas with the viscosity. The values of the stopping power may be more accurate after considering the effect of viscosity. Our results may open up new possibilities to control the interaction of ions with 2D electron gas in the surface of metal or semiconductor heterostructure by variation of the viscosity.
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1 School of Physics, Huazhong University of Science and Technology, Wuhan 430074, China
2 Department of Physics, Wuhan University of Technology, Wuhan 430070, China
3 Institute of Fluid Physics, China Academy of Engineering Physics, Mianyang 621900, China
4 Institute of Applied Physics and Computational Mathematics, Beijing 100094, China
5 College of Mathematics and Physics, Inner Mongolia University for the Nationalities, Tongliao 028043, China