Abstract

The January 2022 Hunga Tonga-Hunga Ha’apai volcanic eruption injected a relatively small amount of sulfur dioxide, but significantly more water into the stratosphere than previously seen in the modern satellite record. Here we show that the large amount of water resulted in large perturbations to stratospheric aerosol evolution. Our climate model simulation reproduces the observed enhanced water vapor at pressure levels ~30 hPa for three months. Compared with a simulation without a water injection, this additional source of water vapor increases hydroxide, which halves the sulfur dioxide lifetime. Subsequent coagulation creates larger sulfate particles that double the stratospheric aerosol optical depth. A seasonal forecast of volcanic plume transport in the southern hemisphere indicates this eruption will greatly enhance the aerosol surface area and water vapor near the polar vortex until at least October 2022, suggesting that there will continue to be an impact of this eruption on the climate system.

Large amounts of water vapour released to the stratosphere during the 2022 Hunga-Tonga hydromagmatic volcanic eruption led to decreased sulfur dioxide aerosol lifetime, increased sulfate particle size and a doubling of stratospheric aerosol optical depth, according to numerical simulations.

Details

Title
Perturbations in stratospheric aerosol evolution due to the water-rich plume of the 2022 Hunga-Tonga eruption
Author
Zhu, Yunqian 1   VIAFID ORCID Logo  ; Bardeen, Charles G. 2 ; Tilmes, Simone 2 ; Mills, Michael J. 2   VIAFID ORCID Logo  ; Wang, Xinyue 2 ; Harvey, V. Lynn 3 ; Taha, Ghassan 4 ; Kinnison, Douglas 2 ; Portmann, Robert W. 5   VIAFID ORCID Logo  ; Yu, Pengfei 6 ; Rosenlof, Karen H. 5   VIAFID ORCID Logo  ; Avery, Melody 7   VIAFID ORCID Logo  ; Kloss, Corinna 8 ; Li, Can 9 ; Glanville, Anne S. 2 ; Millán, Luis 10 ; Deshler, Terry 3 ; Krotkov, Nickolay 11   VIAFID ORCID Logo  ; Toon, Owen B. 12 

 National Center for Atmospheric Research, Atmospheric Chemistry Observations and Modeling Laboratory, Boulder, USA (GRID:grid.57828.30) (ISNI:0000 0004 0637 9680); University of Colorado Boulder, Laboratory for Atmospheric and Space Physics, Boulder, USA (GRID:grid.266190.a) (ISNI:0000000096214564); University of Colorado Cooperative Institute for Research in Environmental Sciences (CIRES) at the NOAA Chemical Sciences Laboratory, Boulder, USA (GRID:grid.510984.1) (ISNI:0000 0004 9410 3069) 
 National Center for Atmospheric Research, Atmospheric Chemistry Observations and Modeling Laboratory, Boulder, USA (GRID:grid.57828.30) (ISNI:0000 0004 0637 9680) 
 University of Colorado Boulder, Laboratory for Atmospheric and Space Physics, Boulder, USA (GRID:grid.266190.a) (ISNI:0000000096214564) 
 Morgan State University, GESTAR II, Baltimore, USA (GRID:grid.260238.d) (ISNI:0000 0001 2224 4258); National Aeronautics and Space Administration, Goddard Space Flight Center, Greenbelt, USA (GRID:grid.238252.c) (ISNI:0000 0001 1456 7559) 
 National Oceanic and Atmospheric Administration, Chemical Sciences Laboratory, Boulder, USA (GRID:grid.3532.7) (ISNI:0000 0001 1266 2261) 
 Jinan University, Institute for Environmental and Climate Research, Guangzhou, China (GRID:grid.258164.c) (ISNI:0000 0004 1790 3548) 
 University of Colorado Cooperative Institute for Research in Environmental Sciences (CIRES) at the NOAA Chemical Sciences Laboratory, Boulder, USA (GRID:grid.510984.1) (ISNI:0000 0004 9410 3069); NASA Langley Research Center, Hampton, USA (GRID:grid.419086.2) (ISNI:0000 0004 0637 6754) 
 CNRS UMR 7328, Université d’Orléans, Laboratoire de Physique et Chimie de l’Environnement et de l’Espace, Orléans, France (GRID:grid.112485.b) (ISNI:0000 0001 0217 6921) 
 National Aeronautics and Space Administration, Goddard Space Flight Center, Greenbelt, USA (GRID:grid.238252.c) (ISNI:0000 0001 1456 7559); University of Maryland, Earth System Science Interdisciplinary Center, College Park, USA (GRID:grid.164295.d) (ISNI:0000 0001 0941 7177) 
10  California Institute of Technology, Jet Propulsion Laboratory, Pasadena, USA (GRID:grid.20861.3d) (ISNI:0000000107068890) 
11  National Aeronautics and Space Administration, Goddard Space Flight Center, Greenbelt, USA (GRID:grid.238252.c) (ISNI:0000 0001 1456 7559) 
12  University of Colorado Boulder, Laboratory for Atmospheric and Space Physics, Boulder, USA (GRID:grid.266190.a) (ISNI:0000000096214564); University of Colorado Boulder, Department of Atmospheric and Oceanic Sciences, Boulder, USA (GRID:grid.266190.a) (ISNI:0000000096214564) 
Publication year
2022
Publication date
Dec 2022
Publisher
Nature Publishing Group
e-ISSN
26624435
Source type
Scholarly Journal
Language of publication
English
ProQuest document ID
2727287524
Copyright
© The Author(s) 2022. This work is published under http://creativecommons.org/licenses/by/4.0/ (the “License”). Notwithstanding the ProQuest Terms and Conditions, you may use this content in accordance with the terms of the License.