Abstract

The properties of superheavy elements probe extremes of physics and chemistry. They are synthesised at accelerator laboratories using nuclear fusion, where two atomic nuclei collide, stick together (capture), then with low probability evolve to a compact superheavy nucleus. The fundamental microscopic mechanisms controlling fusion are not fully understood, limiting predictive capability. Even capture, considered to be the simplest stage of fusion, is not matched by models. Here we show that collisions of 40Ca with 208Pb, experience an ‘explosion’ of mass and charge transfers between the nuclei before capture, with unexpectedly high probability and complexity. Ninety different partitions of the protons and neutrons between the projectile-like and target-like nuclei are observed. Since each is expected to have a different probability of fusion, the early stages of collisions may be crucial in superheavy element synthesis. Our interpretation challenges the current view of fusion, explains both the successes and failures of current capture models, and provides a framework for improved models.

Superheavy nuclei are synthesized in the laboratory through the fusion of lighter nuclei. Here the authors study multinucleon transfer and interactions during the early stages of nuclear fusion in the collision of 40Ca and 208Pb nuclei showing early onset of complexity.

Details

Title
Colliding heavy nuclei take multiple identities on the path to fusion
Author
Cook, Kaitlin J. 1   VIAFID ORCID Logo  ; Rafferty, Dominic C. 2 ; Hinde, David J. 2 ; Simpson, Edward C. 2 ; Dasgupta, Mahananda 2 ; Corradi, Lorenzo 3 ; Evers, Maurits 2 ; Fioretto, Enrico 3 ; Jeung, Dongyun 2   VIAFID ORCID Logo  ; Lobanov, Nikolai 2   VIAFID ORCID Logo  ; Luong, Duc Huy 2 ; Mijatović, Tea 4   VIAFID ORCID Logo  ; Montagnoli, Giovanna 5 ; Stefanini, Alberto M. 3 ; Szilner, Suzana 4 

 The Australian National University, Department of Nuclear Physics and Accelerator Applications, Research School of Physics, Canberra, Australia (GRID:grid.1001.0) (ISNI:0000 0001 2180 7477); Michigan State University, Facility for Rare Isotope Beams, East Lansing, USA (GRID:grid.17088.36) (ISNI:0000 0001 2150 1785) 
 The Australian National University, Department of Nuclear Physics and Accelerator Applications, Research School of Physics, Canberra, Australia (GRID:grid.1001.0) (ISNI:0000 0001 2180 7477) 
 Laboratori Nazionali di Legnaro, Istituto Nazionale di Fisica Nucleare, Legnaro, Italy (GRID:grid.466875.e) (ISNI:0000 0004 1757 5572) 
 Ruđer Bošković Institute, Zagreb, Croatia (GRID:grid.4905.8) (ISNI:0000 0004 0635 7705) 
 Universita di Padova, Dipartimento di Fisica e Astronomia, Padova, Italy (GRID:grid.5608.b) (ISNI:0000 0004 1757 3470) 
Pages
7988
Publication year
2023
Publication date
2023
Publisher
Nature Publishing Group
e-ISSN
20411723
Source type
Scholarly Journal
Language of publication
English
ProQuest document ID
2896129597
Copyright
© The Author(s) 2023. This work is published under http://creativecommons.org/licenses/by/4.0/ (the “License”). Notwithstanding the ProQuest Terms and Conditions, you may use this content in accordance with the terms of the License.