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Abstract
Miniaturized spectrometers have great potential for use in portable optoelectronics and wearable sensors. However, current strategies for miniaturization rely on von Neumann architectures, which separate the spectral sensing, storage, and processing modules spatially, resulting in high energy consumption and limited processing speeds due to the storage-wall problem. Here, we present a miniaturized spectrometer that utilizes a single SnS2/ReSe2 van der Waals heterostructure, providing photodetection, spectrum reconstruction, spectral imaging, long-term image memory, and signal processing capabilities. Interface trap states are found to induce a gate-tunable and wavelength-dependent photogating effect and a non-volatile optoelectronic memory effect. Our approach achieves a footprint of 19 μm, a bandwidth from 400 to 800 nm, a spectral resolution of 5 nm, and a > 104 s long-term image memory. Our single-detector computational spectrometer represents a path beyond von Neumann architectures.
Recent studies have reported miniaturized spectrometers based on van der Waals heterostructures. Here, the authors demonstrate multifunctional SnS2/ReSe2 heterojunction spectrometers providing photodetection, spectrum reconstruction, spectral imaging, long-term image memory, and signal processing capabilities.
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Details
; Cho, Jiung 3 ; Choi, Miri 4
; Ó Coileáin, Cormac 5 ; Hung, Kuan-Ming 6
; Chang, Ching-Ray 7
; Shvets, Igor V. 8 ; Wu, Han-Chun 1
1 Beijing Institute of Technology, School of Physics, Beijing, P. R. China (GRID:grid.43555.32) (ISNI:0000 0000 8841 6246)
2 University of Applied Sciences, Geneva, Switzerland (GRID:grid.510272.3)
3 Korea Basic Science Institute, Western Seoul Cente, Seoul, Republic of Korea (GRID:grid.410885.0) (ISNI:0000 0000 9149 5707); Chung-Ang University, 4726, Seodong-daero, Daedeok-myeon, Department of Advanced Materials Engineering, Anseong-si, Republic of Korea (GRID:grid.254224.7) (ISNI:0000 0001 0789 9563)
4 Korea Basic Science Institute, Chuncheon Center, Chuncheon, Republic of Korea (GRID:grid.410885.0) (ISNI:0000 0000 9149 5707)
5 University of the Bundeswehr Munich, Institute of Physics, Faculty of Electrical Engineering and Information Technology, Neubiberg, Germany (GRID:grid.7752.7) (ISNI:0000 0000 8801 1556)
6 National Kaohsiung University of Science and Technology, Department of Electronics Engineering, Kaohsiung, Taiwan, ROC (GRID:grid.7752.7) (ISNI:0000 0004 6470 0890)
7 Chung Yuan Christian University, Quantum Information Center, Taoyuan, Taiwan, ROC (GRID:grid.411649.f) (ISNI:0000 0004 0532 2121); National Taiwan University, Department of Physics, Taipei, Taiwan, ROC (GRID:grid.19188.39) (ISNI:0000 0004 0546 0241)
8 Trinity College Dublin, Dublin, School of Physics, Dublin 2, Ireland (GRID:grid.8217.c) (ISNI:0000 0004 1936 9705)




