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Abstract
Photoionization can initiate structural reorganization of molecular matter and drive formation of new chemical bonds. Here, we used time-resolved extreme ultraviolet (EUV) pump – EUV probe Coulomb explosion imaging of carbon dioxide dimer ion
In a time-resolved Coulomb explosion imaging study using ultrafast extreme ultraviolet pulses, combined with theoretical simulations, authors reveal unexpected asymmetric rearrangement of carbon dioxide dimer ion, including a CO3 moiety formation.
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1 The Hebrew University of Jerusalem, Institute of Chemistry, Jerusalem, Israel (GRID:grid.9619.7) (ISNI:0000 0004 1937 0538); The Hebrew University of Jerusalem, Fritz Haber Research Center for Molecular Dynamics, Jerusalem, Israel (GRID:grid.9619.7) (ISNI:0000 0004 1937 0538)
2 The Hebrew University of Jerusalem, Institute of Chemistry, Jerusalem, Israel (GRID:grid.9619.7) (ISNI:0000 0004 1937 0538)
3 Max Planck Institute for Nuclear Physics, Heidelberg, Germany (GRID:grid.419604.e) (ISNI:0000 0001 2288 6103)
4 Deutsches Elektronen-Synchrotron DESY, Hamburg, Germany (GRID:grid.7683.a) (ISNI:0000 0004 0492 0453)
5 The Hebrew University of Jerusalem, Institute of Chemistry, Jerusalem, Israel (GRID:grid.9619.7) (ISNI:0000 0004 1937 0538); IISER-Thiruvananthapuram, Kerala, India (GRID:grid.462378.c) (ISNI:0000 0004 1764 2464)