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Abstract
Long-term, high-frequency atmospheric CO2 measurements at multiple sites in Salt Lake City (SLC), Utah, reveal that annual and monthly CO2 variability aligns with a priori estimates of emissions from anthropogenic and biological sources. In this study, we investigate whether short-term fluctuations in anthropogenic emissions, as captured in the Vulcan3 dataset for the United States, can be detected in atmospheric CO2 observations. Specifically, we focus on Thanksgiving holidays, when traffic and energy usage patterns differ from the rest of November. Onroad CO2 emissions exhibit a double peak during weekday morning and evening rush hours but remain relatively low on weekends and Thanksgiving. Interestingly, CO2 mole fractions during Thanksgiving were higher than the rest of November at all SLC monitoring sites, particularly from 2008 to 2013. This increase is partially attributed to elevated energy-related emissions — especially residential sources — and meteorological factors such as weak wind speeds, cold temperature, and a low planetary boundary layer height (PBLH). While CO2 emissions and mole fraction patterns align over time, notable spatial differences exist. For instance, the near-highway site in Murray shows the highest CO2 mole fractions despite low local emissions, suggesting pollution transport via highways and wind advection. Random Forest model-based SHapley Additive exPlanations (SHAP) analysis reveals that onroad emissions dominate CO2 contributions on weekdays and weekends, while energy-related emissions play a larger role during Thanksgiving, alongside meteorological drivers such as wind speed and PBLH. Across six urban cities, CO2 emissions display a consistent pattern: residential and commercial emissions peak during Thanksgiving with substantial year-to-year variability, while onroad emissions peak during weekdays, with minimal variability. These findings highlight that urban CO2 variability is driven by the combined influence of emissions and meteorology, underscoring the need for integrated mitigation strategies. Additionally, multi-site measurements are essential for accurate source attribution and effective policy interventions.
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1 Atmospheric Science Branch, Earth Science Division, NASA Ames Research Center, Moffett Field, CA 94035, United States of America; Bay Area Environmental Research Institute , Moffett Field, CA 94035, United States of America
2 Department of Earth and Planetary Science, University of California , Berkeley, Berkeley, CA 94720, United States of America; Department of Environmental Science, Policy and Management, University of California , Berkeley, Berkeley, CA 94720, United States of America
3 Department of Biology, University of Utah , Salt Lake City, UT 84112, United States of America