Strontium isotope ratios of human hair record intra-city variations in tap water source

Abstract

The oxygen (¹⁸O/¹⁶O) isotope analysis of hair is commonly applied to reconstruct an individual’s residence history. However, region-of-origin as determined from oxygen isotope values (δ¹⁸O) alone is often spatially indistinct. Adding additional geochemical recorders can refine region-of-origin estimates. In this capacity, strontium (⁸⁷Sr/⁸⁶Sr) isotope analysis has attracted increased interest. While ⁸⁷Sr/⁸⁶Sr reflects the influences of local geology, ⁸⁷Sr/⁸⁶Sr of hair includes both external environmental signals as well as the internal dietary indicators. To better understand the impact of these contributions to the spatial signal encoded within ⁸⁷Sr/⁸⁶Sr of hair, human hair was collected from three locations within Salt Lake City, Utah along with the donor’s sex. The ⁸⁷Sr/⁸⁶Sr and δ¹⁸O of hair and local tap water were measured. There were no significant relationships between sex and either δ¹⁸O or ⁸⁷Sr/⁸⁶Sr of hair, nor between collection location and the δ¹⁸O of hair. However, we found significant associations between collection location and ⁸⁷Sr/⁸⁶Sr of hair. These findings suggest that interactions with local water may be an important source of Sr to human hair and that the ⁸⁷Sr/⁸⁶Sr of hair may have the capacity to record differences in ⁸⁷Sr/⁸⁶Sr of tap waters on small spatial scales.