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Abstract
The non-thermal nature of self-propelling colloids offers new insights into non-equilibrium physics. The central mathematical model to describe their trajectories is active Brownian motion, where a particle moves with a constant speed, while randomly changing direction due to rotational diffusion. While several feedback strategies exist to achieve position-dependent velocity, the possibility of spatial and temporal control over rotational diffusion, which is inherently dictated by thermal fluctuations, remains untapped. Here, we decouple rotational diffusion from thermal fluctuations. Using external magnetic fields and discrete-time feedback loops, we tune the rotational diffusivity of active colloids above and below its thermal value at will and explore a rich range of phenomena including anomalous diffusion, directed transport, and localization. These findings add a new dimension to the control of active matter, with implications for a broad range of disciplines, from optimal transport to smart materials.
Active colloidal systems can serve as an enabling platform to study complex out-of-equilibrium physical phenomena. Using a magnetic control with a feedback loop, here the authors program the dynamics of active Brownian particles by updating their rotational diffusion coefficient depending on their locations.
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1 Department of Materials, Laboratory for Soft Materials and Interfaces, Zurich, Switzerland (GRID:grid.5801.c) (ISNI:0000 0001 2156 2780)
2 Department of Materials, Laboratory for Soft Materials and Interfaces, Zurich, Switzerland (GRID:grid.5801.c) (ISNI:0000 0001 2156 2780); Heinrich-Heine University, Institut für Experimentelle Kolloidphysik, Düsseldorf, Germany (GRID:grid.411327.2) (ISNI:0000 0001 2176 9917)
3 University of Gothenburg, Department of Physics, Gothenburg, Sweden (GRID:grid.8761.8) (ISNI:0000 0000 9919 9582)