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Abstract
Glass structures of multicomponent oxide systems (CaO–Al2O3–SiO2) are studied using a simulated pulsed laser with molecular dynamics. The short- and intermediate-range order structures revealed a direct correlation between the transformation of Al(IV) to Al(V), regions of increased density following laser processing, inherent reduction in the average T–O–T (T = Al, Si) angle, and associated elongation of the T–O bonding distance. Variable laser pulse energies were simulated across calcium aluminosilicate glasses with high silica content (50–80%) to identify densification trends attributed to composition and laser energy. High-intensity pulsed laser effects on fictive temperature and shockwave promotion are discussed in detail for their role in glass densification. Laser-induced structural changes are found to be highly dependent on pulse energy and glass chemistry.
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Details
1 Alfred University, Kazuo Inamori School of Engineering, The New York State College of Ceramics, Ultrafast Materials Science and Engineering Laboratory (U-Lab), Alfred, USA (GRID:grid.252018.c) (ISNI:0000 0001 0725 292X)
2 Corning Incorporated, Science and Technology Division, Corning, USA (GRID:grid.417796.a)