Abstract
Highlights
This review summarizes recent progresses in pristine metal–organic frameworks (MOFs), MOF composites, and their derivatives for next-generation rechargeable batteries including lithium–sulfur batteries, lithium–oxygen batteries, sodium-ion batteries, potassium-ion batteries, Zn-ion batteries, and Zn–air batteries.
The design strategies for MOF-based materials as the electrode, separator, and electrolyte are outlined and discussed.
The challenges and development strategies and of MOF-related materials for battery applications are highlighted.
Metal–organic framework (MOF)-based materials with high porosity, tunable compositions, diverse structures, and versatile functionalities provide great scope for next-generation rechargeable battery applications. Herein, this review summarizes recent advances in pristine MOFs, MOF composites, MOF derivatives, and MOF composite derivatives for high-performance sodium-ion batteries, potassium-ion batteries, Zn-ion batteries, lithium–sulfur batteries, lithium–oxygen batteries, and Zn–air batteries in which the unique roles of MOFs as electrodes, separators, and even electrolyte are highlighted. Furthermore, through the discussion of MOF-based materials in each battery system, the key principles for controllable synthesis of diverse MOF-based materials and electrochemical performance improvement mechanisms are discussed in detail. Finally, the major challenges and perspectives of MOFs are also proposed for next-generation battery applications.
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1 Beijing Institute of Technology, Beijing Key Laboratory of Environmental Science and Engineering, School of Materials Science and Engineering, Beijing, People’s Republic of China (GRID:grid.43555.32) (ISNI:0000 0000 8841 6246)
2 Beijing Institute of Technology, Beijing Key Laboratory of Environmental Science and Engineering, School of Materials Science and Engineering, Beijing, People’s Republic of China (GRID:grid.43555.32) (ISNI:0000 0000 8841 6246); Collaborative Innovation Center of Electric Vehicles in Beijing, Beijing, People’s Republic of China (GRID:grid.43555.32) (ISNI:0000 0000 8841 6246); Beijing Institute of Technology, Advanced Technology Research Institute, Jinan, People’s Republic of China (GRID:grid.43555.32) (ISNI:0000 0000 8841 6246)