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Abstract
The measurement and control of light field oscillations enable the study of ultrafast phenomena on sub-cycle time scales. Electro-optic sampling (EOS) is a powerful field characterization approach, in terms of both sensitivity and dynamic range, but it has not reached beyond infrared frequencies. Here, we show the synthesis of a sub-cycle infrared-visible pulse and subsequent complete electric field characterization using EOS. The sampled bandwidth spans from 700 nm to 2700 nm (428 to 110 THz). Tailored electric-field waveforms are generated with a two-channel field synthesizer in the infrared-visible range, with a full-width at half-maximum duration as short as 3.8 fs at a central wavelength of 1.7 µm (176 THz). EOS detection of the complete bandwidth of these waveforms extends it into the visible spectral range. To demonstrate the power of our approach, we use the sub-cycle transients to inject carriers in a thin quartz sample for nonlinear photoconductive field sampling with sub-femtosecond resolution.
A continuum spanning from 300 and 3000 nm is used to synthesize a single-cycle field transient and measure its waveform through electro-optic sampling, speeding up this sensitive technique so that it can access the electric field of visible light.
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1 Max-Planck-Institut für Quantenoptik, Garching, Germany (GRID:grid.450272.6) (ISNI:0000 0001 1011 8465); Fakultät für Physik, Ludwig-Maximilians-Universität, Garching, Germany (GRID:grid.5252.0) (ISNI:0000 0004 1936 973X); University of California, Department of Chemistry, Berkeley, USA (GRID:grid.47840.3f) (ISNI:0000 0001 2181 7878)
2 Max-Planck-Institut für Quantenoptik, Garching, Germany (GRID:grid.450272.6) (ISNI:0000 0001 1011 8465); Fakultät für Physik, Ludwig-Maximilians-Universität, Garching, Germany (GRID:grid.5252.0) (ISNI:0000 0004 1936 973X)
3 Max-Planck-Institut für Quantenoptik, Garching, Germany (GRID:grid.450272.6) (ISNI:0000 0001 1011 8465); Fakultät für Physik, Ludwig-Maximilians-Universität, Garching, Germany (GRID:grid.5252.0) (ISNI:0000 0004 1936 973X); SLAC National Accelerator Laboratory, Menlo Park, USA (GRID:grid.445003.6) (ISNI:0000 0001 0725 7771)
4 Max-Planck-Institut für Quantenoptik, Garching, Germany (GRID:grid.450272.6) (ISNI:0000 0001 1011 8465); Fakultät für Physik, Ludwig-Maximilians-Universität, Garching, Germany (GRID:grid.5252.0) (ISNI:0000 0004 1936 973X); Ultrafast Innovations GmbH, Garching, Germany (GRID:grid.5252.0)
5 Max-Planck-Institut für Quantenoptik, Garching, Germany (GRID:grid.450272.6) (ISNI:0000 0001 1011 8465); CNR NANOTEC Institute of Nanotechnology, via Monteroni, Lecce, Italy (GRID:grid.494551.8) (ISNI:0000 0004 6477 0549)