Real-space nanoimaging of THz polaritons in the topological insulator Bi2Se3

Abstract

Plasmon polaritons in topological insulators attract attention from a fundamental perspective and for potential THz photonic applications. Although polaritons have been observed by THz far-field spectroscopy on topological insulator microstructures, real-space imaging of propagating THz polaritons has been elusive so far. Here, we show spectroscopic THz near-field images of thin Bi₂Se₃ layers (prototypical topological insulators) revealing polaritons with up to 12 times increased momenta as compared to photons of the same energy and decay times of about 0.48 ps, yet short propagation lengths. From the images we determine and analyze the polariton dispersion, showing that the polaritons can be explained by the coupling of THz radiation to various combinations of Dirac and massive carriers at the Bi₂Se₃ surfaces, massive bulk carriers and optical phonons. Our work provides critical insights into the nature of THz polaritons in topological insulators and establishes instrumentation and methodology for imaging of THz polaritons.

The real-space imaging of propagating THz polaritons, coupled light-matter excitations, in topological insulators has been elusive so far. Here, the authors report spectroscopic THz near-field images of the topological insulator Bi₂Se₃ revealing polaritons formed by coupling of THz radiation to optical phonons and various charge carriers.