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Abstract
Combining the superior photovoltaic performance of three-dimensional perovskites and the intrinsic durability of two-dimensional perovskites, the construction of 3D/2D perovskite bilayer heterojunctions is a promising strategy to realize efficient and stable perovskite solar cells, but it is still a challenge to control the phase purity, film thickness, orientation, and crystal structure of 2D perovskites. Now, a solution-processing strategy has overcome this challenge by directly coating a tailored single-crystal 2D perovskite ink on as-prepared 3D perovskite films, resulting in effective, ultra-stable and phase-pure 3D/2D perovskite bilayer heterojunctions.
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Details
1 Fudan University, Department of Materials Science, Institute of Optoelectronics, Shanghai Frontiers Science Research Base of Intelligent Optoelectronics and Perception, Shanghai, China (GRID:grid.8547.e) (ISNI:0000 0001 0125 2443)