Abstract

Finding d-electron heavy fermion states has been an important topic as the diversity in d-electron materials can lead to many exotic Kondo effect-related phenomena or new states of matter such as correlation-driven topological Kondo insulator. Yet, obtaining direct spectroscopic evidence for a d-electron heavy fermion system has been elusive to date. Here, we report the observation of Kondo lattice behavior in an antiferromagnetic metal, FeTe, via angle-resolved photoemission spectroscopy, scanning tunneling spectroscopy and transport property measurements. The Kondo lattice behavior is represented by the emergence of a sharp quasiparticle and Fano-type tunneling spectra at low temperatures. The transport property measurements confirm the low-temperature Fermi liquid behavior and reveal successive coherent-incoherent crossover upon increasing temperature. We interpret the Kondo lattice behavior as a result of hybridization between localized Fe 3dxy and itinerant Te 5pz orbitals. Our observations strongly suggest unusual cooperation between Kondo lattice behavior and long-range magnetic order.

The Kondo hybridization typically occurs in heavy-fermion systems containing f electrons, although recently it has been reported in d-electron systems. Kim et al. report spectroscopic evidence of the Kondo hybridization in FeTe and discuss it role in the mechanism of the magnetic order.

Details

Title
Kondo interaction in FeTe and its potential role in the magnetic order
Author
Kim, Younsik 1 ; Kim, Min-Seok 2 ; Kim, Dongwook 3 ; Kim, Minjae 4 ; Kim, Minsoo 1   VIAFID ORCID Logo  ; Cheng, Cheng-Maw 5   VIAFID ORCID Logo  ; Choi, Joonyoung 6   VIAFID ORCID Logo  ; Jung, Saegyeol 1 ; Lu, Donghui 7   VIAFID ORCID Logo  ; Kim, Jong Hyuk 8 ; Cho, Soohyun 9 ; Song, Dongjoon 1 ; Oh, Dongjin 10   VIAFID ORCID Logo  ; Yu, Li 11   VIAFID ORCID Logo  ; Choi, Young Jai 8   VIAFID ORCID Logo  ; Kim, Hyeong-Do 12 ; Han, Jung Hoon 13 ; Jo, Younjung 6 ; Shim, Ji Hoon 3   VIAFID ORCID Logo  ; Seo, Jungpil 2   VIAFID ORCID Logo  ; Huh, Soonsang 1   VIAFID ORCID Logo  ; Kim, Changyoung 1   VIAFID ORCID Logo 

 Institute for Basic Science, Center for Correlated Electron Systems, Seoul, Korea (GRID:grid.410720.0) (ISNI:0000 0004 1784 4496); Seoul National University, Department of Physics & Astronomy, Seoul, Korea (GRID:grid.31501.36) (ISNI:0000 0004 0470 5905) 
 DGIST, Department of Emerging Materials Science, Daegu, Korea (GRID:grid.417736.0) (ISNI:0000 0004 0438 6721) 
 Pohang University of Science and Technology (POSTECH), Department of Chemistry, Pohang, Korea (GRID:grid.49100.3c) (ISNI:0000 0001 0742 4007) 
 Korea Institute for Advanced Study, Seoul, Korea (GRID:grid.249961.1) (ISNI:0000 0004 0610 5612) 
 National Synchrotron Radiation Research Center, Hsinchu, Taiwan (GRID:grid.410766.2) (ISNI:0000 0001 0749 1496) 
 Kyungpook National University, Department of Physics, Daegu, Korea (GRID:grid.258803.4) (ISNI:0000 0001 0661 1556) 
 SLAC National Accelerator Laboratory, Stanford Synchrotron Radiation Light Source, Menlo Park, USA (GRID:grid.445003.6) (ISNI:0000 0001 0725 7771) 
 Yonsei University, Department of Physics, Seoul, Korea (GRID:grid.15444.30) (ISNI:0000 0004 0470 5454) 
 Chinese Academy of Sciences, Center for Excellence in Superconducting Electronics, State Key Laboratory of Functional Materials for Informatics, Shanghai Institute of Microsystem and Information Technology, Shanghai, China (GRID:grid.9227.e) (ISNI:0000000119573309) 
10  Institute for Basic Science, Center for Correlated Electron Systems, Seoul, Korea (GRID:grid.410720.0) (ISNI:0000 0004 1784 4496); Seoul National University, Department of Physics & Astronomy, Seoul, Korea (GRID:grid.31501.36) (ISNI:0000 0004 0470 5905); Massachusetts Institute of Technology, Department of Physics, Cambridge, USA (GRID:grid.116068.8) (ISNI:0000 0001 2341 2786) 
11  Chinese Academy of Sciences, Beijing National Laboratory for Condensed Matter Physics and Institute of Physics, Beijing, China (GRID:grid.9227.e) (ISNI:0000 0001 1957 3309); University of Chinese Academy of Sciences, School of Physical Sciences, Beijing, China (GRID:grid.410726.6) (ISNI:0000 0004 1797 8419); Songshan Lake Materials Laboratory, Dongguan, China (GRID:grid.511002.7) 
12  Pohang Accelerator Laboratory, XFEL Beamline Division, Pohang, Korea (GRID:grid.15444.30) (ISNI:0000 0004 0632 5770) 
13  Sungkyunkwan University, Department of Physics, Suwon, Korea (GRID:grid.264381.a) (ISNI:0000 0001 2181 989X) 
Pages
4145
Publication year
2023
Publication date
2023
Publisher
Nature Publishing Group
e-ISSN
20411723
Source type
Scholarly Journal
Language of publication
English
ProQuest document ID
2836142541
Copyright
© The Author(s) 2023. corrected publication 2024. This work is published under http://creativecommons.org/licenses/by/4.0/ (the “License”). Notwithstanding the ProQuest Terms and Conditions, you may use this content in accordance with the terms of the License.