Abstract

In this paper, we report an eco-friendly approach for the C(sp2)–H bond selenylation of imidazopyridines and other N-heteroarenes as well as simple arenes at ambient temperature. This new protocol consists of the reaction between (N-hetero)-arenes and the diorganyl-diselenides and trichloroisocyanuric acid (TCCA)-ethanol reagent system. In a short reaction time, the desired selenylated products were obtained regioselectively in good yields, with tolerance for a wide range of functional groups.

Details

Title
Catalyst- and metal-free C(sp2)–H bond selenylation of (N-hetero)-arenes using diselenides and trichloroisocyanuric acid at room temperature
Author
Neto, José S. S. 1 ; Granja, Isis J. A. 2 ; Scheide, Marcos R. 3 ; Franco, Marcelo S. 3 ; Moraes, Cassio A. O. 4 ; Beatriz, Adilson 4 ; de Lima, Dênis P. 4 ; Botteselle, Giancarlo V. 5 ; Frizon, Tiago E. A. 6 ; Saba, Sumbal 2 ; Rafique, Jamal 7 ; Braga, Antonio L. 3 

 Universidade Federal de Santa Catarina–UFSC, Departamento de Química, Florianópolis, Brazil (GRID:grid.411237.2) (ISNI:0000 0001 2188 7235); Universidade Federal de Goiás–UFG, Instituto de Química, Goiânia, Brazil (GRID:grid.411195.9) (ISNI:0000 0001 2192 5801) 
 Universidade Federal de Goiás–UFG, Instituto de Química, Goiânia, Brazil (GRID:grid.411195.9) (ISNI:0000 0001 2192 5801) 
 Universidade Federal de Santa Catarina–UFSC, Departamento de Química, Florianópolis, Brazil (GRID:grid.411237.2) (ISNI:0000 0001 2188 7235) 
 Universidade Federal do Mato Grosso do Sul–UFMS, Instituto de Química, Campo Grande, Brazil (GRID:grid.412352.3) (ISNI:0000 0001 2163 5978) 
 Universidade Estadual do Centro-Oeste–UNICENTRO, Departamento de Química, Guarapuava, Brazil (GRID:grid.412329.f) (ISNI:0000 0001 1581 1066) 
 Universidade Federal de Santa Catarina–UFSC, Araranguá, Brazil (GRID:grid.411237.2) (ISNI:0000 0001 2188 7235) 
 Universidade Federal de Goiás–UFG, Instituto de Química, Goiânia, Brazil (GRID:grid.411195.9) (ISNI:0000 0001 2192 5801); Universidade Federal do Mato Grosso do Sul–UFMS, Instituto de Química, Campo Grande, Brazil (GRID:grid.412352.3) (ISNI:0000 0001 2163 5978) 
Pages
14251
Publication year
2023
Publication date
2023
Publisher
Nature Publishing Group
e-ISSN
20452322
Source type
Scholarly Journal
Language of publication
English
ProQuest document ID
2859399803
Copyright
© The Author(s) 2023. This work is published under http://creativecommons.org/licenses/by/4.0/ (the “License”). Notwithstanding the ProQuest Terms and Conditions, you may use this content in accordance with the terms of the License.