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Abstract
We present a formally exact and simulation-free approach for the normalization of X-ray Thomson scattering (XRTS) spectra based on the f-sum rule of the imaginary-time correlation function (ITCF). Our method works for any degree of collectivity, over a broad range of temperatures, and is applicable even in nonequilibrium situations. In addition to giving us model-free access to electronic correlations, this new approach opens up the intriguing possibility to extract a plethora of physical properties from the ITCF based on XRTS experiments.
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1 Center for Advanced Systems Understanding (CASUS), Görlitz, Germany (GRID:grid.510908.5); Helmholtz-Zentrum Dresden-Rossendorf (HZDR), Dresden, Germany (GRID:grid.40602.30) (ISNI:0000 0001 2158 0612)
2 Lawrence Livermore National Laboratory (LLNL), Livermore, USA (GRID:grid.250008.f) (ISNI:0000 0001 2160 9702)
3 Sandia National Laboratories, Center for Computing Research, Albuquerque, USA (GRID:grid.474520.0) (ISNI:0000 0001 2151 9272)
4 Royal Institute of Technology (KTH), Space and Plasma Physics, Stockholm, Sweden (GRID:grid.5037.1) (ISNI:0000 0001 2158 1746)
5 Center for Advanced Systems Understanding (CASUS), Görlitz, Germany (GRID:grid.510908.5); Helmholtz-Zentrum Dresden-Rossendorf (HZDR), Dresden, Germany (GRID:grid.40602.30) (ISNI:0000 0001 2158 0612); Technische Universität Dresden, Dresden, Germany (GRID:grid.4488.0) (ISNI:0000 0001 2111 7257)
6 Universität Rostock, Institut für Physik, Rostock, Germany (GRID:grid.10493.3f) (ISNI:0000 0001 2185 8338)
7 First Light Fusion, Yarnton, Oxfordshire, UK (GRID:grid.10493.3f) (ISNI:0000 0004 6359 2015)
8 European XFEL, Schenefeld, Germany (GRID:grid.434729.f) (ISNI:0000 0004 0590 2900)
9 Helmholtz-Zentrum Dresden-Rossendorf (HZDR), Dresden, Germany (GRID:grid.40602.30) (ISNI:0000 0001 2158 0612)